It makes no sense to use Po210, which is extremely expensive and even extremely dangerous to handle for the assassinator and would immediately point with the finger at Putin himself. If he wanted to kill Litvinenko, he could have done it much smarter. As far as I could follow, Po210 is only supposed to be the poison, because of it's almost non-detectibility, but not proved. Anyway Russian dissidents die like flies nowadays, creepy times!
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